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Redox-neutral electrochemical decontamination of hypersaline wastewater with excessive know-how readiness degree


  • Chung, M. G., Frank, Ok. A., Pokhrel, Y., Dietz, T. & Liu, J. Pure infrastructure in sustaining international city freshwater ecosystem providers. Nat. Maintain. 4, 1068–1075 (2021).

    Article 

    Google Scholar
     

  • Zhang, X. et al. Managing nitrogen for sustainable improvement. Nature 528, 51–59 (2015).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Panagopoulos, A. & Giannika, V. Comparative techno-economic and environmental evaluation of minimal liquid discharge (MLD) and 0 liquid discharge (ZLD) desalination methods for seawater brine therapy and valorization. Maintain. Power Technol. Assess. 53, 102477 (2022).


    Google Scholar
     

  • Menon, A. Ok., Haechler, I., Kaur, S., Lubner, S. & Prasher, R. S. Enhanced photo voltaic evaporation utilizing a photo-thermal umbrella for wastewater administration. Nat. Maintain. 3, 144–151 (2020).

    Article 

    Google Scholar
     

  • Kumar, A., Phillips, Ok. R., Thiel, G. P., Schröder, U. & Lienhard, J. H. Direct electrosynthesis of sodium hydroxide and hydrochloric acid from brine streams. Nat. Catal. 2, 106–113 (2019).

    Article 
    CAS 

    Google Scholar
     

  • Shehzad, M. A. et al. Shielded goethite catalyst that allows quick water dissociation in bipolar membranes. Nat. Commun. 12, 9 (2021).

    Article 
    CAS 
    PubMed 
    PubMed Central 

    Google Scholar
     

  • Zhang, W. et al. Impression of chloride ions on UV/H2O2 and UV/persulfate superior oxidation processes. Environ. Sci. Technol. 52, 7380–7389 (2018).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Chen, Y. et al. Tip-intensified interfacial microenvironment reconstruction promotes an electrocatalytic chlorine evolution response. ACS Catal. 12, 14376–14386 (2022).

    Article 
    CAS 

    Google Scholar
     

  • Liu, J., Zhang, X. & Li, Y. Photoconversion of chlorinated saline wastewater DBPs in receiving seawater is total a cleansing course of. Environ. Sci. Technol. 51, 58–67 (2017).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Yang, T. et al. Environment friendly degradation of organoarsenic by UV/chlorine therapy: kinetics, mechanism, enhanced arsenic elimination, and cytotoxicity. Environ. Sci. Technol. 55, 2037–2047 (2021).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Rao, U. et al. Structural dependence of reductive defluorination of linear PFAS compounds in a UV/electrochemical system. Environ. Sci. Technol. 54, 10668–10677 (2020).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Guo, Ok., Wu, Z., Chen, C. & Fang, J. UV/chlorine course of: an environment friendly superior oxidation course of with a number of radicals and capabilities in water therapy. Acc. Chem. Res. 55, 286–297 (2022).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Choi, C. et al. Environment friendly electrocatalytic valorization of chlorinated natural water pollutant to ethylene. Nat. Nanotechnol. 18, 160–167 (2023).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Fang, J., Fu, Y. & Shang, C. The roles of reactive species in micropollutant degradation within the UV/free chlorine system. Environ. Sci. Technol. 48, 1859–1868 (2014).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Zhang, J., Zhang, G., Lan, H., Qu, J. & Liu, H. Synergetic hydroxyl radical oxidation with atomic hydrogen discount lowers the organochlorine conversion barrier and potentiates efficient contaminant mineralization. Environ. Sci. Technol. 55, 3296–3304 (2021).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Llorente, M. J., Nguyen, B. H., Kubiak, C. P. & Moeller, Ok. D. Paired electrolysis within the simultaneous manufacturing of artificial intermediates and substrates. J. Am. Chem. Soc. 138, 15110–15113 (2016).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Min, Y. et al. Mimicking reductive dehalogenases for environment friendly electrocatalytic water dechlorination. Nat. Commun. 14, 5134 (2023).

    Article 
    CAS 
    PubMed 
    PubMed Central 

    Google Scholar
     

  • Dwinandha, D., Zhang, B. & Fujii, M. Prediction of response mechanism for OH radical-mediated phenol oxidation utilizing quantum chemical calculation. Chemosphere 291, 132763 (2022).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Atobe, M., Tateno, H. & Matsumura, Y. Purposes of circulate microreactors in electrosynthetic processes. Chem. Rev. 118, 4541–4572 (2018).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Finke, C. E. et al. Enhancing the exercise of oxygen-evolution and chlorine-evolution electro-catalysts by atomic layer deposition of TiO2. Power Environ. Sci. 12, 358–365 (2019).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Karlsson, R. Ok. B. & Cornell, A. Selectivity between oxygen and chlorine evolution within the chlor-alkali and chlorate processes. Chem. Rev. 116, 2982–3028 (2016).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Näslund, L.-Å. et al. The function of TiO2 doping on RuO2-coated electrodes for the water oxidation response. J. Phys. Chem. C 117, 6126–6135 (2013).

    Article 

    Google Scholar
     

  • Jiao, Y., Jiang, H. & Chen, F. RuO2/TiO2/Pt ternary photocatalysts with epitaxial heterojunction and their utility in CO oxidation. ACS Catal. 4, 2249–2257 (2014).

    Article 
    CAS 

    Google Scholar
     

  • Morales-Guio, C. G. et al. Photo voltaic hydrogen manufacturing by amorphous silicon photocathodes coated with a magnetron sputter deposited Mo2C catalyst. J. Am. Chem. Soc. 137, 7035–7038 (2015).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Dong, C. et al. Totally uncovered palladium cluster catalysts allow hydrogen manufacturing from nitrogen heterocycles. Nat. Catal. 5, 485–493 (2022).

    Article 
    CAS 

    Google Scholar
     

  • Xiong, H. et al. Engineering catalyst helps to stabilize PdOx two-dimensional rafts for water-tolerant methane oxidation. Nat. Catal. 4, 830–839 (2021).

    Article 
    CAS 

    Google Scholar
     

  • Ghassemzadeh, L., Peckham, T. J., Weissbach, T., Luo, X. & Holdcroft, S. Selective formation of hydrogen and hydroxyl radicals by electron beam irradiation and their reactivity with perfluorosulfonated acid ionomer. J. Am. Chem. Soc. 135, 15923–15932 (2013).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Xu, B., Chen, Z., Zhang, G. & Wang, Y. On-demand atomic hydrogen provision by exposing electron-rich cobalt websites in an open-framework construction towards superior electrocatalytic nitrate conversion to dinitrogen. Environ. Sci. Technol. 56, 614–623 (2022).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Wang, J. et al. Ambient ammonia synthesis by way of palladium-catalyzed electrohydrogenation of dinitrogen at low overpotential. Nat. Commun. 9, 1795 (2018).

    Article 
    PubMed 
    PubMed Central 

    Google Scholar
     

  • Kakade, B. A., Tamaki, T., Ohashi, H. & Yamaguchi, T. Extremely energetic bimetallic PdPt and CoPt nanocrystals for methanol electro-oxidation. J. Phys. Chem. C 116, 7464–7470 (2012).

    Article 
    CAS 

    Google Scholar
     

  • Zuo, Ok. et al. Electrified water therapy: fundamentals and roles of electrode supplies. Nat. Rev. Mater. 8, 472–490 (2023).

    Article 

    Google Scholar
     

  • Wang, H.-X., Toh, W. L., Tang, B. Y. & Surendranath, Y. Steel surfaces catalyse polarization-dependent hydride switch from H2. Nat. Catal. 6, 351–362 (2023).

    Article 

    Google Scholar
     

  • Sakamoto, H. et al. Photocatalytic dehalogenation of fragrant halides on Ta2O5-supported Pt–Pd bimetallic alloy nanoparticles activated by seen mild. ACS Catal. 7, 5194–5201 (2017).

    Article 
    CAS 

    Google Scholar
     

  • Walter, T. H. et al. Spin trapping in heterogeneous electron switch processes. Can. J. Chem. 60, 1621–1636 (1982).

    Article 
    CAS 

    Google Scholar
     

  • Barroso-Martínez, J. S. et al. Actual-time detection of hydroxyl radical generated at working electrodes by way of redox-active adduct formation utilizing scanning electrochemical microscopy. J. Am. Chem. Soc. 144, 18896–18907 (2022).

    Article 
    PubMed 
    PubMed Central 

    Google Scholar
     

  • Hong, J. et al. Metastable hexagonal close-packed palladium hydride in liquid cell TEM. Nature 603, 631–636 (2022).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Van Buren, J., Prasse, C., Marron, E. L., Skeel, B. & Sedlak, D. L. Ring-cleavage merchandise produced in the course of the preliminary part of oxidative therapy of alkyl-substituted fragrant compounds. Environ. Sci. Technol. 54, 8352–8361 (2020).

    Article 
    PubMed 
    PubMed Central 

    Google Scholar
     

  • Wang, Y., Wei, Y., Track, W., Chen, C. & Zhao, J. Photocatalytic hydrodehalogenation for the elimination of halogenated fragrant contaminants. ChemCatChem 11, 258–268 (2019).

    Article 
    CAS 

    Google Scholar
     

  • Yang, J. et al. CO2-mediated organocatalytic chlorine evolution below industrial circumstances. Nature 617, 519–523 (2023).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Over, H. Floor chemistry of ruthenium dioxide in heterogeneous catalysis and electrocatalysis: from elementary to utilized analysis. Chem. Rev. 112, 3356–3426 (2012).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Lin, J. et al. Shielding impact allows quick ion switch by means of nanoporous membrane for extremely energy-efficient electrodialysis. Nat. Water 1, 725–735 (2023).

    Article 

    Google Scholar
     

  • Butler, J. D., Parkerton, T. F., Redman, A. D., Letinski, D. J. & Cooper, Ok. R. Assessing aromatic-hydrocarbon toxicity to fish youth phases utilizing passive-dosing strategies and target-lipid and chemical-activity fashions. Environ. Sci. Technol. 50, 8305–8315 (2016).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Stinn, C. & Allanore, A. Selective sulfidation of metallic compounds. Nature 602, 78–83 (2022).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Zabaniotou, A. Redesigning a bioenergy sector in EU within the transition to round waste-based bioeconomy—a multidisciplinary overview. J. Clear. Prod. 177, 197–206 (2018).

    Article 

    Google Scholar
     

  • Andrew, R. M. International CO2 emissions from cement manufacturing. Earth Syst. Sci. Knowledge 10, 195–217 (2018).

    Article 

    Google Scholar
     

  • Zhao, C., Dao, R., Wang, Y., Yao, J. & Li, H. A DFT investigation exploring the affect of lone electron pair on hyperfine buildings of N-centered radicals. Chem. Phys. 517, 13–23 (2019).

    Article 
    CAS 

    Google Scholar
     

  • Houriez, C., Ferre, N., Siri, D., Tordo, P. & Masella, M. Assessing the accuracy of a QM/MM//MD mixed protocol to compute spectromagnetic properties of polyfunctional nitroxides in answer. Theor. Chem. Acc. 131, 1240 (2012).

  • Yamaguchi, M. DFT calculation of isotropic hyperfine coupling constants of spin adducts of 5,5-dimethyl-1-pyrroline-N-oxide in benzene and water. Comput. Theor. Chem. 1104, 24–31 (2017).

    Article 
    CAS 

    Google Scholar
     

  • Cohen, A. J., Mori-Sánchez, P. & Yang, W. Challenges for density purposeful concept. Chem. Rev. 112, 289–320 (2012).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Gaussian 16 rev. C.01 (Gaussian, Inc., 2016).

  • Zhang, G. & Liu, H. Supply information for “Redox-neutral electrochemical decontamination of hypersaline wastewater with excessive know-how readiness degree”. figshare https://doi.org/10.6084/m9.figshare.25390759 (2024).

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